Abstract
Substitution of Sb in FeSb2 by less than 0.5% of Te induces a transition from a correlated semiconductor to an unconventional metal with large effective charge carrier mass m*. Spanning the entire range of the semiconductor-metal crossover, we observed an almost constant enhancement of the measured thermopower compared to that estimated by the classical theory of electron diffusion. Using the latter for a quantitative description one has to employ an enhancement factor of 10-30. Our observations point to the importance of electron-electron correlations in the thermal transport of FeSb2, and suggest a route to design thermoelectric materials for cryogenic applications.
| Original language | English |
|---|---|
| Article number | 072105 |
| Journal | Applied Physics Letters |
| Volume | 98 |
| Issue number | 7 |
| DOIs | |
| State | Published - 14 Feb 2011 |
| Externally published | Yes |
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