Ultralong Rutile TiO2 Nanowire Arrays for Highly Efficient Dye-Sensitized Solar Cells

Hailiang Li; Qingjiang Yu; Yuewu Huang; Cuiling Yu; Renzhi Li; Jinzhong Wang; Fengyun Guo; Shujie Jiao; Shiyong Gao; Yong Zhang; Xitian Zhang; Peng Wang; Liancheng Zhao

doi:10.1021/acsami.6b01508

Ultralong Rutile TiO₂ Nanowire Arrays for Highly Efficient Dye-Sensitized Solar Cells

Hailiang Li
, Qingjiang Yu^*
, Yuewu Huang
, Cuiling Yu
, Renzhi Li
, Jinzhong Wang
, Fengyun Guo
, Shujie Jiao
, Shiyong Gao
, Yong Zhang
, Xitian Zhang
, Peng Wang
, Liancheng Zhao

^*Corresponding author for this work

Harbin Institute of Technology
CAS - Changchun Institute of Applied Chemistry
Harbin Normal University

Research output: Contribution to journal › Article › peer-review

58 Scopus citations

Abstract

Vertically aligned rutile TiO₂ nanowire arrays (NWAs) with lengths of ∼44 μm have been successfully synthesized on transparent, conductive fluorine-doped tin oxide (FTO) glass by a facile one-step solvothermal method. The length and wire-to-wire distance of NWAs can be controlled by adjusting the ethanol content in the reaction solution. By employing optimized rutile TiO₂ NWAs for dye-sensitized solar cells (DSCs), a remarkable power conversion efficiency (PCE) of 8.9% is achieved. Moreover, in combination with a light-scattering layer, the performance of a rutile TiO₂ NWAs based DSC can be further enhanced, reaching an impressive PCE of 9.6%, which is the highest efficiency for rutile TiO₂ NWA based DSCs so far.

Original language	English
Pages (from-to)	13384-13391
Number of pages	8
Journal	ACS Applied Materials and Interfaces
Volume	8
Issue number	21
DOIs	https://doi.org/10.1021/acsami.6b01508
State	Published - 1 Jun 2016
Externally published	Yes

Keywords

TiO
charge recombination
dye-sensitized solar cells
nanowire arrays
solvothermal synthesis

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10.1021/acsami.6b01508

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@article{5880d9736d73473582ebf0e5114e6950,

title = "Ultralong Rutile TiO2 Nanowire Arrays for Highly Efficient Dye-Sensitized Solar Cells",

abstract = "Vertically aligned rutile TiO2 nanowire arrays (NWAs) with lengths of ∼44 μm have been successfully synthesized on transparent, conductive fluorine-doped tin oxide (FTO) glass by a facile one-step solvothermal method. The length and wire-to-wire distance of NWAs can be controlled by adjusting the ethanol content in the reaction solution. By employing optimized rutile TiO2 NWAs for dye-sensitized solar cells (DSCs), a remarkable power conversion efficiency (PCE) of 8.9\% is achieved. Moreover, in combination with a light-scattering layer, the performance of a rutile TiO2 NWAs based DSC can be further enhanced, reaching an impressive PCE of 9.6\%, which is the highest efficiency for rutile TiO2 NWA based DSCs so far.",

keywords = "TiO, charge recombination, dye-sensitized solar cells, nanowire arrays, solvothermal synthesis",

author = "Hailiang Li and Qingjiang Yu and Yuewu Huang and Cuiling Yu and Renzhi Li and Jinzhong Wang and Fengyun Guo and Shujie Jiao and Shiyong Gao and Yong Zhang and Xitian Zhang and Peng Wang and Liancheng Zhao",

note = "Publisher Copyright: {\textcopyright} 2016 American Chemical Society.",

year = "2016",

month = jun,

day = "1",

doi = "10.1021/acsami.6b01508",

language = "英语",

volume = "8",

pages = "13384--13391",

journal = "ACS Applied Materials and Interfaces",

issn = "1944-8244",

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TY - JOUR

T1 - Ultralong Rutile TiO2 Nanowire Arrays for Highly Efficient Dye-Sensitized Solar Cells

AU - Li, Hailiang

AU - Yu, Qingjiang

AU - Huang, Yuewu

AU - Yu, Cuiling

AU - Li, Renzhi

AU - Wang, Jinzhong

AU - Guo, Fengyun

AU - Jiao, Shujie

AU - Gao, Shiyong

AU - Zhang, Yong

AU - Zhang, Xitian

AU - Wang, Peng

AU - Zhao, Liancheng

PY - 2016/6/1

Y1 - 2016/6/1

N2 - Vertically aligned rutile TiO2 nanowire arrays (NWAs) with lengths of ∼44 μm have been successfully synthesized on transparent, conductive fluorine-doped tin oxide (FTO) glass by a facile one-step solvothermal method. The length and wire-to-wire distance of NWAs can be controlled by adjusting the ethanol content in the reaction solution. By employing optimized rutile TiO2 NWAs for dye-sensitized solar cells (DSCs), a remarkable power conversion efficiency (PCE) of 8.9% is achieved. Moreover, in combination with a light-scattering layer, the performance of a rutile TiO2 NWAs based DSC can be further enhanced, reaching an impressive PCE of 9.6%, which is the highest efficiency for rutile TiO2 NWA based DSCs so far.

AB - Vertically aligned rutile TiO2 nanowire arrays (NWAs) with lengths of ∼44 μm have been successfully synthesized on transparent, conductive fluorine-doped tin oxide (FTO) glass by a facile one-step solvothermal method. The length and wire-to-wire distance of NWAs can be controlled by adjusting the ethanol content in the reaction solution. By employing optimized rutile TiO2 NWAs for dye-sensitized solar cells (DSCs), a remarkable power conversion efficiency (PCE) of 8.9% is achieved. Moreover, in combination with a light-scattering layer, the performance of a rutile TiO2 NWAs based DSC can be further enhanced, reaching an impressive PCE of 9.6%, which is the highest efficiency for rutile TiO2 NWA based DSCs so far.

KW - TiO

KW - charge recombination

KW - dye-sensitized solar cells

KW - nanowire arrays

KW - solvothermal synthesis

UR - https://www.scopus.com/pages/publications/84973402385

U2 - 10.1021/acsami.6b01508

DO - 10.1021/acsami.6b01508

M3 - 文章

AN - SCOPUS:84973402385

SN - 1944-8244

VL - 8

SP - 13384

EP - 13391

JO - ACS Applied Materials and Interfaces

JF - ACS Applied Materials and Interfaces

IS - 21

ER -

Ultralong Rutile TiO₂ Nanowire Arrays for Highly Efficient Dye-Sensitized Solar Cells

Abstract

Keywords

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