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Three-Dimensional Wide-Bandwidth Quantum Energy Truncation Terahertz Coherence Tomography

  • Pengfei Zhu
  • , Hai Zhang*
  • , Stefano Sfarra
  • , Fabrizio Sarasini
  • , Xavier Maldague
  • , Andreas Mandelis*
  • *Corresponding author for this work
  • Université Laval
  • University of L'Aquila
  • University of Rome La Sapienza
  • University of Toronto

Research output: Contribution to journalArticlepeer-review

Abstract

We report a quantum energy truncation terahertz coherence tomography technique that enables highly localized extraction of molecular-species-specific THz responses. The method exploits resonant photon loss when the emitter THz energy matches molecular vibration quanta. Reflected THz radiation is recorded and mapped into depth-coded image sequences, from which subsurface structural information and molecular fingerprints are retrieved to construct three-dimensional tomograms. This approach resolves major limitations of conventional continuous-wave (CW) THz imaging—namely, its lack of spectroscopic specificity and dependence on angular scanning—by directly correlating molecular excitation spectra with depth information. As a result, quantum energy truncation terahertz coherence tomography enables rapid, three-dimensional THz imaging with selective sensitivity to discrete molecular quantum energy transitions, providing new opportunities for nondestructive characterization of material refractive indices, molecular composition, and subsurface structures.

Original languageEnglish
Article number026901
JournalPhysical Review Letters
Volume137
Issue number2
DOIs
StatePublished - 10 Jul 2026

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