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The effects of hydrothermal temperature on the photocatalytic performance of ZnIn2S4 for hydrogen generation under visible light irradiation

  • Fei Tian
  • , Rongshu Zhu*
  • , Kelin Song
  • , Minli Niu
  • , Feng Ouyang
  • , Gang Cao
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

A series of ZnIn2S4 photocatalysts were successfully synthesized using the hydrothermal method with different hydrothermal temperatures (120, 140, 160, 180, and 200 °C) and characterized by various analysis techniques, such as UV-vis, XRD, SEM, BET and PL. The results indicated that these photocatalysts had a similar band gap. The hydrothermal temperature had a huge influence on the properties of the photocatalysts such as the BET surface area, the total pore volume, the average pore diameter, the defects and the morphology. The photocatalytic activities of ZnIn2S4 were evaluated based on photocatalytic hydrogen production from water under visible-light irradiation. The activity order is attributed to the coefficient of the surface morphology and the surface defects. The hydrogen production efficiency achieved the best when the hydrothermal temperature was 160 °C. On the basis of the characterization of the catalysts, the effects of the hydrothermal temperature on the photocatalytic activity of ZnIn2S4 were discussed.

Original languageEnglish
Pages (from-to)645-650
Number of pages6
JournalMaterials Research Bulletin
Volume70
DOIs
StatePublished - 12 Jun 2015
Externally publishedYes

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

Keywords

  • A. Chalcogenides
  • A. Semiconductors
  • B. Solvothermal
  • D. Catalytic properties
  • D. Crystal structure

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