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Synthesis and characterization of 4-phenylethynylphthalic anhydride

  • Harbin Institute of Technology
  • Heilongjiang Province Environmental Monitoring Center

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

4-phenylethynylphthalic anhydride (4-PEPA) was synthesized by the palladium/copper catalyzed Sonogashira coupling reaction between phenylacetylene and 4-bromophthalic anhydride. The yield achieved 85.48%. The single crystal of 4-PEPA was grown and crystallized by solvent diffusion method. The structure of the compound was characterized by single crystal X-ray diffracttion method, UV-vis, 1H NMR, 13C NMR and FTIR. All characterizations above demonstrated the structure of 4-PEPA. HPLC gave the purity achieving 96.62%. TG-DSC was used to investigate the thermal stability of the compound. Vibrational frequencies of 4-PEPA calculated using the density functional theory (DFT/B3LYP) method with the 6-31G(d) basis sets were in good agreement with experimental values.

Original languageEnglish
Title of host publicationAdvanced Engineering Materials III
Pages1769-1772
Number of pages4
DOIs
StatePublished - 2013
Event3rd International Conference on Advanced Engineering Materials and Technology, AEMT 2013 - Zhangjiajie, China
Duration: 11 May 201312 May 2013

Publication series

NameAdvanced Materials Research
Volume750-752
ISSN (Print)1022-6680

Conference

Conference3rd International Conference on Advanced Engineering Materials and Technology, AEMT 2013
Country/TerritoryChina
CityZhangjiajie
Period11/05/1312/05/13

Keywords

  • 4-phenylethynylphthalic anhydride
  • DFT
  • End-capping reagent
  • Polyimide
  • Single crystal

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