Abstract
The importance of electronic structure evolutions and reconstitutions is widely acknowledged for strongly correlated systems. The precise effect of pressurized Fermi surface topology on metallization and superconductivity is a much-debated topic. In this work, an evolution from insulating to metallic behavior, followed by a superconducting transition, is systematically investigated in SnS2 under high pressure. In-situ X-ray diffraction measurements show the stability of the trigonal structure under compression. Interestingly, a Lifshitz transition, which has an important bearing on the metallization and superconductivity, is identified by the first-principles calculations between 35 and 40 GPa. Our findings provide a unique playground for exploring the relationship of electronic structure, metallization, and superconductivity under high pressure without crystal structural collapse.
| Original language | English |
|---|---|
| Pages (from-to) | 9404-9410 |
| Number of pages | 7 |
| Journal | Journal of Physical Chemistry Letters |
| Volume | 13 |
| Issue number | 40 |
| DOIs | |
| State | Published - 13 Oct 2022 |
| Externally published | Yes |
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