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Selective detection of trace carbon monoxide at room temperature based on CuO nanosheets exposed to (111) crystal facets

  • Yuanyuan Wu
  • , Ji Li
  • , Mingsong Lv
  • , Xianfa Zhang
  • , Rui Gao
  • , Chuanyu Guo
  • , Xiaoli Cheng
  • , Xin Zhou
  • , Yingming Xu*
  • , Shan Gao
  • , Zoltán Major
  • , Lihua Huo
  • *Corresponding author for this work
  • Heilongjiang University
  • School of Chemistry and Chemical Engineering, Harbin Institute of Technology
  • Johannes Kepler University Linz

Research output: Contribution to journalArticlepeer-review

Abstract

In recent years, carbon monoxide (CO) intoxication incidents occur frequently, and the sensitive detection of CO is particularly significant. At present, most reported carbon monoxide (CO) sensors meet the disadvantage of high working temperature. It is always a challenge to realize the sensitive detection of carbon monoxide at room temperature. In this study, CuO nanosheets exposed more (111) active crystal facets and oxygen vacancy defects were synthesized by a simple and environmentally friendly one-step hydrothermal method. The sensor has good comprehensive gas sensing performance, compared with other sensors that can detect CO at room temperature. The response value to 100 ppm CO at room temperature is as high as 39.6. In addition, it also has excellent selectivity, low detection limit (100 ppb), good reproducibility, moisture resistance and long-term stability (60 days). This excellent gas sensing performance is attributed to the special structural characteristics of 2D materials and the synergistic effect of more active crystal facets exposed on the crystal surface and oxygen vacancy defects. Therefore, it is expected to become a promising sensitive material for rapid and accurate detection of trace CO gas under low energy consumption, reduce the risk of poisoning, and then effectively protect human life safety.

Original languageEnglish
Article number130041
JournalJournal of Hazardous Materials
Volume442
DOIs
StatePublished - 15 Jan 2023
Externally publishedYes

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

Keywords

  • Carbon monoxide
  • CuO nanosheets
  • Exposed CuO (111) active crystal facets
  • Oxygen vacancy defects
  • Room temperature detection

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