Real-time mass-spectrometric screening of droplet-scale electrochemical reactions

Hong Zhang; Kai Yu; Na Li; Jing He; Lina Qiao; Ming Li; Yingying Wang; Dongmei Zhang; Jie Jiang; Richard N. Zare

doi:10.1039/c8an00957k

Real-time mass-spectrometric screening of droplet-scale electrochemical reactions

Hong Zhang
, Kai Yu
, Na Li
, Jing He
, Lina Qiao
, Ming Li
, Yingying Wang
, Dongmei Zhang
, Jie Jiang^*
, Richard N. Zare

^*Corresponding author for this work

School of Marine Science and Technology

School of Marine Science and Technology, Harbin Institute of Technology Weihai
Harbin Institute of Technology
National Institute of Metrology China
Stanford University

Research output: Contribution to journal › Article › peer-review

19 Scopus citations

Abstract

A droplet-scale, real-time electrochemical reaction screening platform based on droplet spray ionization mass spectrometry (DSI-MS) has been developed. The N,N-dimethylaniline (DMA) radical cation with a half-life of microseconds was readily detected by MS during the electrooxidation of DMA, and the subsequent reactions were followed in real time for minutes.

Original language	English
Pages (from-to)	4247-4250
Number of pages	4
Journal	Analyst
Volume	143
Issue number	18
DOIs	https://doi.org/10.1039/c8an00957k
State	Published - 21 Sep 2018

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10.1039/c8an00957k

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title = "Real-time mass-spectrometric screening of droplet-scale electrochemical reactions",

abstract = "A droplet-scale, real-time electrochemical reaction screening platform based on droplet spray ionization mass spectrometry (DSI-MS) has been developed. The N,N-dimethylaniline (DMA) radical cation with a half-life of microseconds was readily detected by MS during the electrooxidation of DMA, and the subsequent reactions were followed in real time for minutes.",

author = "Hong Zhang and Kai Yu and Na Li and Jing He and Lina Qiao and Ming Li and Yingying Wang and Dongmei Zhang and Jie Jiang and Zare, \{Richard N.\}",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry.",

year = "2018",

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day = "21",

doi = "10.1039/c8an00957k",

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T1 - Real-time mass-spectrometric screening of droplet-scale electrochemical reactions

AU - Zhang, Hong

AU - Yu, Kai

AU - Li, Na

AU - He, Jing

AU - Qiao, Lina

AU - Li, Ming

AU - Wang, Yingying

AU - Zhang, Dongmei

AU - Jiang, Jie

AU - Zare, Richard N.

PY - 2018/9/21

Y1 - 2018/9/21

N2 - A droplet-scale, real-time electrochemical reaction screening platform based on droplet spray ionization mass spectrometry (DSI-MS) has been developed. The N,N-dimethylaniline (DMA) radical cation with a half-life of microseconds was readily detected by MS during the electrooxidation of DMA, and the subsequent reactions were followed in real time for minutes.

AB - A droplet-scale, real-time electrochemical reaction screening platform based on droplet spray ionization mass spectrometry (DSI-MS) has been developed. The N,N-dimethylaniline (DMA) radical cation with a half-life of microseconds was readily detected by MS during the electrooxidation of DMA, and the subsequent reactions were followed in real time for minutes.

UR - https://www.scopus.com/pages/publications/85053379935

U2 - 10.1039/c8an00957k

DO - 10.1039/c8an00957k

M3 - 文章

C2 - 30027961

AN - SCOPUS:85053379935

SN - 0003-2654

VL - 143

SP - 4247

EP - 4250

JO - Analyst

JF - Analyst

IS - 18

ER -

Real-time mass-spectrometric screening of droplet-scale electrochemical reactions

Abstract

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