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Quantum beats of vibrational modes in both the low and high wavenumber regions studied by fs-CARS

  • Yanqiang Yang*
  • , Xin Du
  • , Xing He
  • , Yunfei Song
  • , Yang Wang
  • , Yuqiang Liu
  • , Lilin Jiang
  • , Mingfu Zhang
  • *Corresponding author for this work
  • Harbin Institute of Technology
  • Harbin University of Commerce

Research output: Contribution to journalArticlepeer-review

Abstract

We have studied the quantum beats of vibrational modes in different phase samples by employing femtosecond time-resolved coherent anti-Stokes Raman scattering (fs-CARS) technique. The temporal chirped white-light continuum (WLC) is used for the Stokes pulse, we have achieved the selective excitation of vibrational modes in both the low and high wavenumber regions without complicated laser system, and observed quantum coherence between vibrational modes. This work is of special significance to enhance our understanding of quantum coherence and develop the applications of quantum technologies.

Original languageEnglish
Pages (from-to)1324-1327
Number of pages4
JournalOptics and Laser Technology
Volume44
Issue number5
DOIs
StatePublished - Jul 2012

Keywords

  • CARS
  • Quantum beat
  • Time-resolved

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