Pushing CO2-philic membrane performance to the limit by designing semi-interpenetrating networks (SIPN) for sustainable CO2 separations

Xu Jiang; Songwei Li; Lu Shao

doi:10.1039/c6ee03566c

Pushing CO₂-philic membrane performance to the limit by designing semi-interpenetrating networks (SIPN) for sustainable CO₂ separations

Xu Jiang
, Songwei Li
, Lu Shao^*

^*Corresponding author for this work

School of Chemistry and Chemical Engineering, Harbin Institute of Technology

Research output: Contribution to journal › Article › peer-review

196 Scopus citations

Abstract

Semi-interpenetrating network (SIPN) membranes with unprecedentedly high CO₂ permeability were designed and synthesized simply through one-step, UV-induced radical polymerization. The in situ embedment of linear polyethylene glycol as a "CO₂ transport promoter" in membranes can dramatically enhance both CO₂ solubility and diffusivity to push SIPN membrane performance beyond Robeson's upper bound line (2008). This extremely facile performance-manipulating strategy establishes our CO₂-philic SIPN membranes as an exciting platform for sustainable CO₂ separations.

Original language	English
Pages (from-to)	1339-1344
Number of pages	6
Journal	Energy and Environmental Science
Volume	10
Issue number	6
DOIs	https://doi.org/10.1039/c6ee03566c
State	Published - Jun 2017
Externally published	Yes

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Access to Document

10.1039/c6ee03566c

Cite this

@article{3aa491c8cc26404eb52eaabb918fa284,

title = "Pushing CO2-philic membrane performance to the limit by designing semi-interpenetrating networks (SIPN) for sustainable CO2 separations",

abstract = "Semi-interpenetrating network (SIPN) membranes with unprecedentedly high CO2 permeability were designed and synthesized simply through one-step, UV-induced radical polymerization. The in situ embedment of linear polyethylene glycol as a {"}CO2 transport promoter{"} in membranes can dramatically enhance both CO2 solubility and diffusivity to push SIPN membrane performance beyond Robeson's upper bound line (2008). This extremely facile performance-manipulating strategy establishes our CO2-philic SIPN membranes as an exciting platform for sustainable CO2 separations.",

author = "Xu Jiang and Songwei Li and Lu Shao",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry 2017.",

year = "2017",

month = jun,

doi = "10.1039/c6ee03566c",

language = "英语",

volume = "10",

pages = "1339--1344",

journal = "Energy and Environmental Science",

issn = "1754-5692",

publisher = "Royal Society of Chemistry",

number = "6",

}

TY - JOUR

T1 - Pushing CO2-philic membrane performance to the limit by designing semi-interpenetrating networks (SIPN) for sustainable CO2 separations

AU - Jiang, Xu

AU - Li, Songwei

AU - Shao, Lu

PY - 2017/6

Y1 - 2017/6

N2 - Semi-interpenetrating network (SIPN) membranes with unprecedentedly high CO2 permeability were designed and synthesized simply through one-step, UV-induced radical polymerization. The in situ embedment of linear polyethylene glycol as a "CO2 transport promoter" in membranes can dramatically enhance both CO2 solubility and diffusivity to push SIPN membrane performance beyond Robeson's upper bound line (2008). This extremely facile performance-manipulating strategy establishes our CO2-philic SIPN membranes as an exciting platform for sustainable CO2 separations.

AB - Semi-interpenetrating network (SIPN) membranes with unprecedentedly high CO2 permeability were designed and synthesized simply through one-step, UV-induced radical polymerization. The in situ embedment of linear polyethylene glycol as a "CO2 transport promoter" in membranes can dramatically enhance both CO2 solubility and diffusivity to push SIPN membrane performance beyond Robeson's upper bound line (2008). This extremely facile performance-manipulating strategy establishes our CO2-philic SIPN membranes as an exciting platform for sustainable CO2 separations.

UR - https://www.scopus.com/pages/publications/85018966986

U2 - 10.1039/c6ee03566c

DO - 10.1039/c6ee03566c

M3 - 文章

AN - SCOPUS:85018966986

SN - 1754-5692

VL - 10

SP - 1339

EP - 1344

JO - Energy and Environmental Science

JF - Energy and Environmental Science

IS - 6

ER -

Pushing CO₂-philic membrane performance to the limit by designing semi-interpenetrating networks (SIPN) for sustainable CO₂ separations

Abstract

UN SDGs

Access to Document

Other files and links

Fingerprint

Cite this