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Pressure tuning of thermoelectric performance in FeNbSb

  • Hong Jie Pang
  • , Hao Yu
  • , Liu Cheng Chen
  • , Chen Guang Fu
  • , Tie Jun Zhu
  • , Xiao Jia Chen*
  • *Corresponding author for this work
  • Center for High Pressure Science & Technology Advanced Research
  • Zhejiang University
  • Max Planck Institute for Chemical Physics of Solids

Research output: Contribution to journalArticlepeer-review

Abstract

Thermoelectric materials offer an ideal solution for the global energy crisis and environmental pollution as which can directly convert waste heat into electricity. From the view of device application, achieving large figure of merit zT at room temperature is highly desirable. Here, we choose a half-Heusler compound FeNb0.8Ti0.2Sb with a maximum zT of 1.1 at 1100 K as an example. By using the developed techniques for the high-pressure measurements, we investigate the potential of pressure to tune the thermoelectric performance at room temperature. An obvious improvement of zT by about 62.5 % is achieved at 4 GPa. A pressure-induced electronic topological transition is proposed to contribute to such an improvement. This study points to a promising avenue to enhance the zT of half-Heusler compounds.

Original languageEnglish
Pages (from-to)1224-1230
Number of pages7
JournalJournal of Alloys and Compounds
Volume805
DOIs
StatePublished - 15 Oct 2019
Externally publishedYes

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 12 - Responsible Consumption and Production
    SDG 12 Responsible Consumption and Production

Keywords

  • High pressure
  • Raman spectroscopy
  • Transport properties
  • thermoelectricity

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