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Pressure dependence of degenerate four-wave mixing in SO2: effect of the thermal gratings

  • Shiming Shi
  • , Deying Chen
  • , Qike Zheng
  • , Maria Person
  • , Qizong Qin
  • Fudan University

Research output: Contribution to journalArticlepeer-review

Abstract

The degenerate four wave mixing (DFWM) spectrum of the A(1A2) ← X(1A1) and B(1B1) ← X(1A1) transitions of SO2 in the 299.5-305 nm region is presented. It has been found that the DFWM signal intensities are proportional to the cube of laser intensity and the square of SO2 pressure. The DFWM signal increases dramatically with the pressure of N2 as a buffer gas. The enhancement of the DFWM signal can be mainly attributed to the thermal grating contribution.

Original languageEnglish
Pages (from-to)167-176
Number of pages10
JournalLaser Chemistry
Volume18
Issue number4
DOIs
StatePublished - 2000
Externally publishedYes

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