Preparation of fluoride adsorbent by resource utilization of carbide slag from industrial waste

Yuanchuan Ren; Jia Tong; Guangfei Qu; Ping Ning; Nanqi Ren; Chaoneng Zhang; Fenghui Wu; Yuyi Yang; Xiuping Chen; Zuolian Wang; Yan Hu; Jun Wang; Ping Lu

doi:10.1016/j.jece.2022.108632

Preparation of fluoride adsorbent by resource utilization of carbide slag from industrial waste

Yuanchuan Ren
, Jia Tong
, Guangfei Qu
, Ping Ning
, Nanqi Ren
, Chaoneng Zhang
, Fenghui Wu
, Yuyi Yang
, Xiuping Chen
, Zuolian Wang
, Yan Hu
, Jun Wang
, Ping Lu

Kunming University of Science and Technology
National Regional Engineering Research Center-NCW
School of Environment, Harbin Institute of Technology

Research output: Contribution to journal › Article › peer-review

14 Scopus citations

Abstract

A high performance fluoride adsorbent was prepared for the removal of fluoride from industrial wastewater by calcination and polyacrylic acid impregnation. Through batch experiments, the removal capacity of the adsorbent for fluorine and the influence of key factors (calcination temperature, dosage of polyacrylic acid, pH, initial fluorine concentration and dosage of adsorbent) on the efficiency of the adsorbent for fluoride removal was investigated. The maximum adsorption capacity and removal of efficiency were 98.61 mg/g and 98.7%, respectively. The adsorption kinetics and isotherm studies showed that the pseudo second order model and Langmuir isotherm model fitted this adsorption process better. Moreover, the mechanism of F- removal by CS, C-CS, PAA@C-CS were further analyzed by SEM, EDS, XRD and FTIR. F- in wastewater were found to be adsorbed on the surface of adsorbent through electrostatic interaction, ion exchange and surface coordination. Recovery is achieved by desorption of the adsorbent material by NaOH (0.1 M). As a highly resourced and eco-friendly adsorbent for removal of F- from industrial wastewater, PAA@C-CS has a promising application for controlling industrial water pollution.

Original language	English
Article number	108632
Journal	Journal of Environmental Chemical Engineering
Volume	10
Issue number	6
DOIs	https://doi.org/10.1016/j.jece.2022.108632
State	Published - Dec 2022
Externally published	Yes

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 12 Responsible Consumption and Production
SDG 13 Climate Action

Keywords

Adsorption
Fluoride
Industrial solid waste
Industrial waste water
Resource utilization

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10.1016/j.jece.2022.108632

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@article{b45f9c6fc889416cb491769ffe7bec76,

title = "Preparation of fluoride adsorbent by resource utilization of carbide slag from industrial waste",

abstract = "A high performance fluoride adsorbent was prepared for the removal of fluoride from industrial wastewater by calcination and polyacrylic acid impregnation. Through batch experiments, the removal capacity of the adsorbent for fluorine and the influence of key factors (calcination temperature, dosage of polyacrylic acid, pH, initial fluorine concentration and dosage of adsorbent) on the efficiency of the adsorbent for fluoride removal was investigated. The maximum adsorption capacity and removal of efficiency were 98.61 mg/g and 98.7\%, respectively. The adsorption kinetics and isotherm studies showed that the pseudo second order model and Langmuir isotherm model fitted this adsorption process better. Moreover, the mechanism of F- removal by CS, C-CS, PAA@C-CS were further analyzed by SEM, EDS, XRD and FTIR. F- in wastewater were found to be adsorbed on the surface of adsorbent through electrostatic interaction, ion exchange and surface coordination. Recovery is achieved by desorption of the adsorbent material by NaOH (0.1 M). As a highly resourced and eco-friendly adsorbent for removal of F- from industrial wastewater, PAA@C-CS has a promising application for controlling industrial water pollution.",

keywords = "Adsorption, Fluoride, Industrial solid waste, Industrial waste water, Resource utilization",

author = "Yuanchuan Ren and Jia Tong and Guangfei Qu and Ping Ning and Nanqi Ren and Chaoneng Zhang and Fenghui Wu and Yuyi Yang and Xiuping Chen and Zuolian Wang and Yan Hu and Jun Wang and Ping Lu",

note = "Publisher Copyright: {\textcopyright} 2022 Elsevier Ltd.",

year = "2022",

month = dec,

doi = "10.1016/j.jece.2022.108632",

language = "英语",

volume = "10",

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TY - JOUR

T1 - Preparation of fluoride adsorbent by resource utilization of carbide slag from industrial waste

AU - Ren, Yuanchuan

AU - Tong, Jia

AU - Qu, Guangfei

AU - Ning, Ping

AU - Ren, Nanqi

AU - Zhang, Chaoneng

AU - Wu, Fenghui

AU - Yang, Yuyi

AU - Chen, Xiuping

AU - Wang, Zuolian

AU - Hu, Yan

AU - Wang, Jun

AU - Lu, Ping

PY - 2022/12

Y1 - 2022/12

N2 - A high performance fluoride adsorbent was prepared for the removal of fluoride from industrial wastewater by calcination and polyacrylic acid impregnation. Through batch experiments, the removal capacity of the adsorbent for fluorine and the influence of key factors (calcination temperature, dosage of polyacrylic acid, pH, initial fluorine concentration and dosage of adsorbent) on the efficiency of the adsorbent for fluoride removal was investigated. The maximum adsorption capacity and removal of efficiency were 98.61 mg/g and 98.7%, respectively. The adsorption kinetics and isotherm studies showed that the pseudo second order model and Langmuir isotherm model fitted this adsorption process better. Moreover, the mechanism of F- removal by CS, C-CS, PAA@C-CS were further analyzed by SEM, EDS, XRD and FTIR. F- in wastewater were found to be adsorbed on the surface of adsorbent through electrostatic interaction, ion exchange and surface coordination. Recovery is achieved by desorption of the adsorbent material by NaOH (0.1 M). As a highly resourced and eco-friendly adsorbent for removal of F- from industrial wastewater, PAA@C-CS has a promising application for controlling industrial water pollution.

AB - A high performance fluoride adsorbent was prepared for the removal of fluoride from industrial wastewater by calcination and polyacrylic acid impregnation. Through batch experiments, the removal capacity of the adsorbent for fluorine and the influence of key factors (calcination temperature, dosage of polyacrylic acid, pH, initial fluorine concentration and dosage of adsorbent) on the efficiency of the adsorbent for fluoride removal was investigated. The maximum adsorption capacity and removal of efficiency were 98.61 mg/g and 98.7%, respectively. The adsorption kinetics and isotherm studies showed that the pseudo second order model and Langmuir isotherm model fitted this adsorption process better. Moreover, the mechanism of F- removal by CS, C-CS, PAA@C-CS were further analyzed by SEM, EDS, XRD and FTIR. F- in wastewater were found to be adsorbed on the surface of adsorbent through electrostatic interaction, ion exchange and surface coordination. Recovery is achieved by desorption of the adsorbent material by NaOH (0.1 M). As a highly resourced and eco-friendly adsorbent for removal of F- from industrial wastewater, PAA@C-CS has a promising application for controlling industrial water pollution.

KW - Adsorption

KW - Fluoride

KW - Industrial solid waste

KW - Industrial waste water

KW - Resource utilization

UR - https://www.scopus.com/pages/publications/85139866085

U2 - 10.1016/j.jece.2022.108632

DO - 10.1016/j.jece.2022.108632

M3 - 文章

AN - SCOPUS:85139866085

SN - 2213-2929

VL - 10

JO - Journal of Environmental Chemical Engineering

JF - Journal of Environmental Chemical Engineering

IS - 6

M1 - 108632

ER -

Preparation of fluoride adsorbent by resource utilization of carbide slag from industrial waste

Abstract

UN SDGs

Keywords

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