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Hardness and elastic modulus profiles of hybrid coatings

  • Harbin Institute of Technology
  • Universidad Nacional de Mar del Plata

Research output: Contribution to journalArticlepeer-review

Abstract

Instrumented-indentation testing (IIT) provided with a continuous stiffness measurement (CSM) technique was employed to measure hardness and elastic modulus profiles of thin organic/inorganic hybrid coatings on glass surfaces. Hybrids were synthesized by the hydrolytic condensation of (3- methacryloxypropyl) trimethoxysilane (MPMS) or vinyltrimethoxysilane (VMS), with 5-30 wt% tetraethoxysilane (TEOS), in the presence of formic acid. Coatings of 600-800 nm on glass substrates were obtained by dip-coating solutions of these hybrids with benzoyl peroxide (BPO) addition, and curing in an oven following a thermal cycle up to 120°C. Both hardness and elastic modulus showed a maximum value close to the surface, followed by a plateau and a significant increase at higher penetrations. Hybrids based on MPMS and 20-30 wt% TEOS exhibited a good combination of intrinsic values of hardness (0.50 GPa) and brittle index (0.06-0.07), that makes them suitable for coatings of plastic substrates.

Original languageEnglish
Pages (from-to)41-46
Number of pages6
JournalJournal of Sol-Gel Science and Technology
Volume34
Issue number1
DOIs
StatePublished - Apr 2005

Keywords

  • Brittle index
  • Continuous stiffness measurement (CSM)
  • Elastic modulus
  • Hardness
  • Hybrid coatings
  • Instrumented-indentation testing (IIT)
  • Ormosils

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