Enhancement of a two-photon-induced reaction in solution using light-harvesting gold nanodimer structures

Botao Wu; Kosei Ueno; Yukie Yokota; Kai Sun; Heping Zeng; Hiroaki Misawa

doi:10.1021/jz300370b

Enhancement of a two-photon-induced reaction in solution using light-harvesting gold nanodimer structures

Botao Wu
, Kosei Ueno
, Yukie Yokota
, Kai Sun
, Heping Zeng
, Hiroaki Misawa^*

^*Corresponding author for this work

Hokkaido University
East China Normal University
Japan Science and Technology Agency

Research output: Contribution to journal › Article › peer-review

43 Scopus citations

Abstract

We performed a quantitative analysis of plasmon-assisted two-photon photochromic reactions on light-harvesting gold nanodimer structures. Our strategy for the quantitative analysis of two-photon-induced photochemical reactions on gold nanostructures is using not only a confined photochemical reaction chamber but also a solution system. The strong intensification of near-field light at the nanogap positions on gold nanodimer pairs promoted two-photon absorption by a closed-form diarylethene derivative, resulting in highly efficient photochromic conversion to the open-form structure.

Original language	English
Pages (from-to)	1443-1447
Number of pages	5
Journal	Journal of Physical Chemistry Letters
Volume	3
Issue number	11
DOIs	https://doi.org/10.1021/jz300370b
State	Published - 7 Jun 2012
Externally published	Yes

Access to Document

10.1021/jz300370b

Cite this

@article{ec2248de1c34491d8ee5a08f41ed45bc,

title = "Enhancement of a two-photon-induced reaction in solution using light-harvesting gold nanodimer structures",

abstract = "We performed a quantitative analysis of plasmon-assisted two-photon photochromic reactions on light-harvesting gold nanodimer structures. Our strategy for the quantitative analysis of two-photon-induced photochemical reactions on gold nanostructures is using not only a confined photochemical reaction chamber but also a solution system. The strong intensification of near-field light at the nanogap positions on gold nanodimer pairs promoted two-photon absorption by a closed-form diarylethene derivative, resulting in highly efficient photochromic conversion to the open-form structure.",

author = "Botao Wu and Kosei Ueno and Yukie Yokota and Kai Sun and Heping Zeng and Hiroaki Misawa",

year = "2012",

month = jun,

day = "7",

doi = "10.1021/jz300370b",

language = "英语",

volume = "3",

pages = "1443--1447",

journal = "Journal of Physical Chemistry Letters",

issn = "1948-7185",

publisher = "American Chemical Society",

number = "11",

}

TY - JOUR

T1 - Enhancement of a two-photon-induced reaction in solution using light-harvesting gold nanodimer structures

AU - Wu, Botao

AU - Ueno, Kosei

AU - Yokota, Yukie

AU - Sun, Kai

AU - Zeng, Heping

AU - Misawa, Hiroaki

PY - 2012/6/7

Y1 - 2012/6/7

N2 - We performed a quantitative analysis of plasmon-assisted two-photon photochromic reactions on light-harvesting gold nanodimer structures. Our strategy for the quantitative analysis of two-photon-induced photochemical reactions on gold nanostructures is using not only a confined photochemical reaction chamber but also a solution system. The strong intensification of near-field light at the nanogap positions on gold nanodimer pairs promoted two-photon absorption by a closed-form diarylethene derivative, resulting in highly efficient photochromic conversion to the open-form structure.

AB - We performed a quantitative analysis of plasmon-assisted two-photon photochromic reactions on light-harvesting gold nanodimer structures. Our strategy for the quantitative analysis of two-photon-induced photochemical reactions on gold nanostructures is using not only a confined photochemical reaction chamber but also a solution system. The strong intensification of near-field light at the nanogap positions on gold nanodimer pairs promoted two-photon absorption by a closed-form diarylethene derivative, resulting in highly efficient photochromic conversion to the open-form structure.

UR - https://www.scopus.com/pages/publications/84861898386

U2 - 10.1021/jz300370b

DO - 10.1021/jz300370b

M3 - 文章

AN - SCOPUS:84861898386

SN - 1948-7185

VL - 3

SP - 1443

EP - 1447

JO - Journal of Physical Chemistry Letters

JF - Journal of Physical Chemistry Letters

IS - 11

ER -

Enhancement of a two-photon-induced reaction in solution using light-harvesting gold nanodimer structures

Abstract

Access to Document

Other files and links

Fingerprint

Cite this