Skip to main navigation Skip to search Skip to main content

Enhanced superconductivity near a pressure-induced quantum critical point of strongly coupled charge density wave order in 2H-Pd0.05TaSe2

  • Yeahan Sur
  • , Dong Hyeon Gim
  • , Dilip Bhoi
  • , Dong Hyun Jang
  • , Keizo Murata
  • , Jia Wei Hu
  • , Kai Zhang
  • , Zi Yu Cao
  • , Viktor V. Struzhkin
  • , Xiao Jia Chen
  • , Kee Hoon Kim*
  • *Corresponding author for this work
  • Seoul National University
  • Center for High Pressure Science & Technology Advanced Research
  • University of Houston

Research output: Contribution to journalArticlepeer-review

Abstract

Interplay between charge density wave (CDW) order and superconductivity (SC) in quasi-two-dimensional materials remains poorly understood due to their diverse experimental varieties. Here, we investigate the pressure-dependent electrical transport and Raman scattering spectra of 2H-Pd0.05TaSe2, which exhibits a CDW transition at TCDW = 115 K and a superconducting transition at Tc = 2.6 K at ambient pressure conditions. As pressure increases, TCDW, identified by the resistivity anomaly, shifts towards lower temperatures and approaches zero at a critical pressure of Pc ~ 21.5 GPa. At this critical pressure, both Tc and upper critical field Hc2 reach their maximum values of ~ 8.5 K and ~ 6.4 T, respectively. Analysis of the Raman scattering spectra demonstrates that increasing pressure systematically suppresses both the two-phonon spectral weight above TCDW and the CDW amplitudon energies below TCDW, leading to their simultaneous disappearance at Pc. These observations provide direct evidence for the formation of a CDW quantum critical point (QCP) at Pc, indicating that charge and lattice fluctuations associated with the QCP of strongly coupled CDW order may enhance SC in pressurized 2H-Pd0.05TaSe2.

Original languageEnglish
Article number8
JournalNPG Asia Materials
Volume17
Issue number1
DOIs
StatePublished - Dec 2025
Externally publishedYes

Fingerprint

Dive into the research topics of 'Enhanced superconductivity near a pressure-induced quantum critical point of strongly coupled charge density wave order in 2H-Pd0.05TaSe2'. Together they form a unique fingerprint.

Cite this