Energy storage performance of sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 films

Jinxin Gu; Qiu Sun; Xiangqun Chen; Ying Song; Yilun Tang; Dongbo Wang; Ping Qu

doi:10.3390/cryst9110575

Energy storage performance of sandwich structured Pb(Zr_0.4Ti_0.6)O₃/BaZr_0.2Ti_0.8O₃/Pb(Zr_0.4Ti_0.6)O₃ films

Jinxin Gu
, Qiu Sun^*
, Xiangqun Chen
, Ying Song
, Yilun Tang
, Dongbo Wang
, Ping Qu

^*Corresponding author for this work

School of Chemistry and Chemical Engineering, Harbin Institute of Technology
Harbin Institute of Technology
School of Energy Science and Engineering, Harbin Institute of Technology

Research output: Contribution to journal › Article › peer-review

17 Scopus citations

Abstract

We reported a sandwich structured Pb(Zr_0.4Ti_0.6)O₃/BaZr_0.2T_i0.8O₃/Pb(Zr_0.4Ti_0.6)O₃ (PZT/BZT/PZT) film fabricated by using the sol–gel method, which was dense and uniform with a unique perovskite structure. The PZT/BZT/PZT films displayed high dielectric constants up to 1722.45 at the frequency of 10 kHz. Additionally, the enhanced energy storage density of 39.27 J·cm⁻³ was achieved at room temperature and 2.00 MV/cm, which was higher than that of the individual BaZr_0.2T_i0.8O₃ film (21.28 J·cm⁻³). Furthermore, the energy storage density and efficiency of PZT/BZT/PZT film increased slightly with the increasing temperature from −140 °C to 200 °C. This work proves the feasibility and effectiveness of a sandwich structure in improving dielectric, leakage, and energy storage performances, providing a new paradigm for high-energy–density dielectrics applications.

Original language	English
Article number	575
Journal	Crystals
Volume	9
Issue number	11
DOIs	https://doi.org/10.3390/cryst9110575
State	Published - Nov 2019
Externally published	Yes

Keywords

Dielectric properties
Energy storage
Sandwich structure
Thin films

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@article{1acfc3526b6344fbb36200ea8cd51a9a,

title = "Energy storage performance of sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 films",

abstract = "We reported a sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 (PZT/BZT/PZT) film fabricated by using the sol–gel method, which was dense and uniform with a unique perovskite structure. The PZT/BZT/PZT films displayed high dielectric constants up to 1722.45 at the frequency of 10 kHz. Additionally, the enhanced energy storage density of 39.27 J·cm−3 was achieved at room temperature and 2.00 MV/cm, which was higher than that of the individual BaZr0.2Ti0.8O3 film (21.28 J·cm−3). Furthermore, the energy storage density and efficiency of PZT/BZT/PZT film increased slightly with the increasing temperature from −140 °C to 200 °C. This work proves the feasibility and effectiveness of a sandwich structure in improving dielectric, leakage, and energy storage performances, providing a new paradigm for high-energy–density dielectrics applications.",

keywords = "Dielectric properties, Energy storage, Sandwich structure, Thin films",

author = "Jinxin Gu and Qiu Sun and Xiangqun Chen and Ying Song and Yilun Tang and Dongbo Wang and Ping Qu",

note = "Publisher Copyright: {\textcopyright} 2019 by the authors.",

year = "2019",

month = nov,

doi = "10.3390/cryst9110575",

language = "英语",

volume = "9",

journal = "Crystals",

issn = "2073-4352",

publisher = "Multidisciplinary Digital Publishing Institute (MDPI)",

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TY - JOUR

T1 - Energy storage performance of sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 films

AU - Gu, Jinxin

AU - Sun, Qiu

AU - Chen, Xiangqun

AU - Song, Ying

AU - Tang, Yilun

AU - Wang, Dongbo

AU - Qu, Ping

PY - 2019/11

Y1 - 2019/11

N2 - We reported a sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 (PZT/BZT/PZT) film fabricated by using the sol–gel method, which was dense and uniform with a unique perovskite structure. The PZT/BZT/PZT films displayed high dielectric constants up to 1722.45 at the frequency of 10 kHz. Additionally, the enhanced energy storage density of 39.27 J·cm−3 was achieved at room temperature and 2.00 MV/cm, which was higher than that of the individual BaZr0.2Ti0.8O3 film (21.28 J·cm−3). Furthermore, the energy storage density and efficiency of PZT/BZT/PZT film increased slightly with the increasing temperature from −140 °C to 200 °C. This work proves the feasibility and effectiveness of a sandwich structure in improving dielectric, leakage, and energy storage performances, providing a new paradigm for high-energy–density dielectrics applications.

AB - We reported a sandwich structured Pb(Zr0.4Ti0.6)O3/BaZr0.2Ti0.8O3/Pb(Zr0.4Ti0.6)O3 (PZT/BZT/PZT) film fabricated by using the sol–gel method, which was dense and uniform with a unique perovskite structure. The PZT/BZT/PZT films displayed high dielectric constants up to 1722.45 at the frequency of 10 kHz. Additionally, the enhanced energy storage density of 39.27 J·cm−3 was achieved at room temperature and 2.00 MV/cm, which was higher than that of the individual BaZr0.2Ti0.8O3 film (21.28 J·cm−3). Furthermore, the energy storage density and efficiency of PZT/BZT/PZT film increased slightly with the increasing temperature from −140 °C to 200 °C. This work proves the feasibility and effectiveness of a sandwich structure in improving dielectric, leakage, and energy storage performances, providing a new paradigm for high-energy–density dielectrics applications.

KW - Dielectric properties

KW - Energy storage

KW - Sandwich structure

KW - Thin films

UR - https://www.scopus.com/pages/publications/85074494535

U2 - 10.3390/cryst9110575

DO - 10.3390/cryst9110575

M3 - 文章

AN - SCOPUS:85074494535

SN - 2073-4352

VL - 9

JO - Crystals

JF - Crystals

IS - 11

M1 - 575

ER -

Energy storage performance of sandwich structured Pb(Zr_0.4Ti_0.6)O₃/BaZr_0.2Ti_0.8O₃/Pb(Zr_0.4Ti_0.6)O₃ films

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