Electric-field-induced strain effects on the magnetization of a P r0.67 S r0.33Mn O3 film

Bangmin Zhang; Cheng Jun Sun; Weiming Lü; T. Venkatesan; Myung Geun Han; Yimei Zhu; Jingsheng Chen; Gan Moog Chow

doi:10.1103/PhysRevB.91.174431

Electric-field-induced strain effects on the magnetization of a P r0.67 S r0.33Mn O3 film

Bangmin Zhang
, Cheng Jun Sun
, Weiming Lü
, T. Venkatesan
, Myung Geun Han
, Yimei Zhu
, Jingsheng Chen
, Gan Moog Chow^*

^*Corresponding author for this work

National University of Singapore
United States Department of Energy
Brookhaven National Laboratory Condensed Matter Physics and Materials Science Department

Research output: Contribution to journal › Article › peer-review

7 Scopus citations

Abstract

The electric-field control of magnetic properties of Pr0.67Sr0.33MnO3 (PSMO) film on piezoelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMNT) substrate was investigated. The piezoelectric response of the PMNT substrate to the electric field produced strain that was coupled to the PSMO film. The in-plane compressive (tensile) strain increased (decreased) the magnetization. The change of magnetic moment was associated with the Mn ions. First-principles simulations showed that the strain-induced electronic redistribution of the two eg orbitals (3dz2 and 3dx2-y2) of Mn ions was responsible for the change of magnetic moment. This work demonstrates that the magnetoelectric effect in manganite/piezoelectric heterostructures originates from the change in eg orbital occupancy of Mn ions induced by strain rather than the interfacial effect.

Original language	English
Article number	174431
Journal	Physical Review B - Condensed Matter and Materials Physics
Volume	91
Issue number	17
DOIs	https://doi.org/10.1103/PhysRevB.91.174431
State	Published - 26 May 2015
Externally published	Yes

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title = "Electric-field-induced strain effects on the magnetization of a P r0.67 S r0.33Mn O3 film",

abstract = "The electric-field control of magnetic properties of Pr0.67Sr0.33MnO3 (PSMO) film on piezoelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMNT) substrate was investigated. The piezoelectric response of the PMNT substrate to the electric field produced strain that was coupled to the PSMO film. The in-plane compressive (tensile) strain increased (decreased) the magnetization. The change of magnetic moment was associated with the Mn ions. First-principles simulations showed that the strain-induced electronic redistribution of the two eg orbitals (3dz2 and 3dx2-y2) of Mn ions was responsible for the change of magnetic moment. This work demonstrates that the magnetoelectric effect in manganite/piezoelectric heterostructures originates from the change in eg orbital occupancy of Mn ions induced by strain rather than the interfacial effect.",

author = "Bangmin Zhang and Sun, \{Cheng Jun\} and Weiming L{\"u} and T. Venkatesan and Han, \{Myung Geun\} and Yimei Zhu and Jingsheng Chen and Chow, \{Gan Moog\}",

note = "Publisher Copyright: {\textcopyright} 2015 American Physical Society.",

year = "2015",

month = may,

day = "26",

doi = "10.1103/PhysRevB.91.174431",

language = "英语",

volume = "91",

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TY - JOUR

T1 - Electric-field-induced strain effects on the magnetization of a P r0.67 S r0.33Mn O3 film

AU - Zhang, Bangmin

AU - Sun, Cheng Jun

AU - Lü, Weiming

AU - Venkatesan, T.

AU - Han, Myung Geun

AU - Zhu, Yimei

AU - Chen, Jingsheng

AU - Chow, Gan Moog

PY - 2015/5/26

Y1 - 2015/5/26

N2 - The electric-field control of magnetic properties of Pr0.67Sr0.33MnO3 (PSMO) film on piezoelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMNT) substrate was investigated. The piezoelectric response of the PMNT substrate to the electric field produced strain that was coupled to the PSMO film. The in-plane compressive (tensile) strain increased (decreased) the magnetization. The change of magnetic moment was associated with the Mn ions. First-principles simulations showed that the strain-induced electronic redistribution of the two eg orbitals (3dz2 and 3dx2-y2) of Mn ions was responsible for the change of magnetic moment. This work demonstrates that the magnetoelectric effect in manganite/piezoelectric heterostructures originates from the change in eg orbital occupancy of Mn ions induced by strain rather than the interfacial effect.

AB - The electric-field control of magnetic properties of Pr0.67Sr0.33MnO3 (PSMO) film on piezoelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMNT) substrate was investigated. The piezoelectric response of the PMNT substrate to the electric field produced strain that was coupled to the PSMO film. The in-plane compressive (tensile) strain increased (decreased) the magnetization. The change of magnetic moment was associated with the Mn ions. First-principles simulations showed that the strain-induced electronic redistribution of the two eg orbitals (3dz2 and 3dx2-y2) of Mn ions was responsible for the change of magnetic moment. This work demonstrates that the magnetoelectric effect in manganite/piezoelectric heterostructures originates from the change in eg orbital occupancy of Mn ions induced by strain rather than the interfacial effect.

UR - https://www.scopus.com/pages/publications/84930200209

U2 - 10.1103/PhysRevB.91.174431

DO - 10.1103/PhysRevB.91.174431

M3 - 文章

AN - SCOPUS:84930200209

SN - 1098-0121

VL - 91

JO - Physical Review B - Condensed Matter and Materials Physics

JF - Physical Review B - Condensed Matter and Materials Physics

IS - 17

M1 - 174431

ER -

Electric-field-induced strain effects on the magnetization of a P r0.67 S r0.33Mn O3 film

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