Constructing stable solid electrolyte interfaces and facilitating Li transport via an electrolyte additive for lithium metal batteries

Meng Li; Zeren Zhou; Qixian Zhang; Yixiang Zhang; Wei Han; Qiaoyan Lin; Lishuang Fan

doi:10.1039/d5cc04166j

Constructing stable solid electrolyte interfaces and facilitating Li transport via an electrolyte additive for lithium metal batteries

Meng Li
, Zeren Zhou
, Qixian Zhang^*
, Yixiang Zhang
, Wei Han^*
, Qiaoyan Lin
, Lishuang Fan^*

^*Corresponding author for this work

School of Chemistry and Chemical Engineering, Harbin Institute of Technology
Shanghai University
TaiZhou University

Research output: Contribution to journal › Article › peer-review

3 Scopus citations

Abstract

Herein, we propose N-methyl-N-(trimethylsilyl) trifluoroacetamide (MSTFA) as an electrolyte additive. MSTFA enters the solvation structure and participates in the formation of a stable SEI/CEI. An electrolyte containing MSTFA makes the Li‖Li cell cycle stably for 400 cycles, while the LiFePO₄‖Li cell maintained 93.6% capacity retention after 500 cycles at 5C.

Original language	English
Journal	Chemical Communications
DOIs	https://doi.org/10.1039/d5cc04166j
State	Accepted/In press - 2025
Externally published	Yes

Access to Document

10.1039/d5cc04166j

Cite this

@article{547ecec41e13475ea7c70b60d777a6a1,

title = "Constructing stable solid electrolyte interfaces and facilitating Li transport via an electrolyte additive for lithium metal batteries",

abstract = "Herein, we propose N-methyl-N-(trimethylsilyl) trifluoroacetamide (MSTFA) as an electrolyte additive. MSTFA enters the solvation structure and participates in the formation of a stable SEI/CEI. An electrolyte containing MSTFA makes the Li‖Li cell cycle stably for 400 cycles, while the LiFePO4‖Li cell maintained 93.6\% capacity retention after 500 cycles at 5C.",

author = "Meng Li and Zeren Zhou and Qixian Zhang and Yixiang Zhang and Wei Han and Qiaoyan Lin and Lishuang Fan",

note = "Publisher Copyright: {\textcopyright} 2025 The Royal Society of Chemistry.",

year = "2025",

doi = "10.1039/d5cc04166j",

language = "英语",

journal = "Chemical Communications",

issn = "1359-7345",

publisher = "Royal Society of Chemistry",

}

TY - JOUR

T1 - Constructing stable solid electrolyte interfaces and facilitating Li transport via an electrolyte additive for lithium metal batteries

AU - Li, Meng

AU - Zhou, Zeren

AU - Zhang, Qixian

AU - Zhang, Yixiang

AU - Han, Wei

AU - Lin, Qiaoyan

AU - Fan, Lishuang

PY - 2025

Y1 - 2025

N2 - Herein, we propose N-methyl-N-(trimethylsilyl) trifluoroacetamide (MSTFA) as an electrolyte additive. MSTFA enters the solvation structure and participates in the formation of a stable SEI/CEI. An electrolyte containing MSTFA makes the Li‖Li cell cycle stably for 400 cycles, while the LiFePO4‖Li cell maintained 93.6% capacity retention after 500 cycles at 5C.

AB - Herein, we propose N-methyl-N-(trimethylsilyl) trifluoroacetamide (MSTFA) as an electrolyte additive. MSTFA enters the solvation structure and participates in the formation of a stable SEI/CEI. An electrolyte containing MSTFA makes the Li‖Li cell cycle stably for 400 cycles, while the LiFePO4‖Li cell maintained 93.6% capacity retention after 500 cycles at 5C.

UR - https://www.scopus.com/pages/publications/105018587261

U2 - 10.1039/d5cc04166j

DO - 10.1039/d5cc04166j

M3 - 文章

C2 - 40980869

AN - SCOPUS:105018587261

SN - 1359-7345

JO - Chemical Communications

JF - Chemical Communications

ER -

Constructing stable solid electrolyte interfaces and facilitating Li transport via an electrolyte additive for lithium metal batteries

Abstract

Access to Document

Other files and links

Fingerprint

Cite this