A symmetrical solid oxide fuel cell prepared by dry-pressing and impregnating methods

Xingbao Zhu; Zhe Lü; Bo Wei; Xiqiang Huang; Yaohui Zhang; Wenhui Su

doi:10.1016/j.jpowsour.2010.07.055

A symmetrical solid oxide fuel cell prepared by dry-pressing and impregnating methods

Xingbao Zhu^*
, Zhe Lü
, Bo Wei
, Xiqiang Huang
, Yaohui Zhang
, Wenhui Su

^*Corresponding author for this work

School of Physics

Harbin Institute of Technology
CAS - International Center for Material Physics

Research output: Contribution to journal › Article › peer-review

78 Scopus citations

Abstract

In this study, a simple and cost-effective dry-pressing method has been used to fabricate a symmetrical solid oxide fuel cell (SOFC) where the dense yttria-stabilized zirconia (YSZ) electrolyte film is sandwiched between two symmetrical porous YSZ layers in which La_0.75Sr_0.25Cr _0.5Mn_0.5O_3-δ (LSCM) based anode and cathode are incorporated using wet impregnation techniques. The maximum power densities (P_max) of a single cell with 32 wt.% LSCM impregnated YSZ anode and cathode reach 333 and 265 mW cm^-2 at 900 °C in dry H₂ and CH₄, respectively. The cell performance is further improved with additional impregnation of a small amount of Sm-doped CeO ₂ (SDC) or Ni. When 6 wt.% Ni as catalyst is added to both the anode and cathode, P_max values of 559 and 547 mW cm^-2 can be achieved, which are better than with SDC. The effect of Ni on the cathode performance is also investigated by impedance spectra analysis.

Original language	English
Pages (from-to)	729-733
Number of pages	5
Journal	Journal of Power Sources
Volume	196
Issue number	2
DOIs	https://doi.org/10.1016/j.jpowsour.2010.07.055
State	Published - 15 Jan 2011

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

Dry-pressing
Nickel/ceria catalyst
Perovskite oxide
Symmetrical solid oxide fuel cells
Wet impregnation

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10.1016/j.jpowsour.2010.07.055

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title = "A symmetrical solid oxide fuel cell prepared by dry-pressing and impregnating methods",

abstract = "In this study, a simple and cost-effective dry-pressing method has been used to fabricate a symmetrical solid oxide fuel cell (SOFC) where the dense yttria-stabilized zirconia (YSZ) electrolyte film is sandwiched between two symmetrical porous YSZ layers in which La0.75Sr0.25Cr 0.5Mn0.5O3-δ (LSCM) based anode and cathode are incorporated using wet impregnation techniques. The maximum power densities (Pmax) of a single cell with 32 wt.\% LSCM impregnated YSZ anode and cathode reach 333 and 265 mW cm-2 at 900 °C in dry H2 and CH4, respectively. The cell performance is further improved with additional impregnation of a small amount of Sm-doped CeO 2 (SDC) or Ni. When 6 wt.\% Ni as catalyst is added to both the anode and cathode, Pmax values of 559 and 547 mW cm-2 can be achieved, which are better than with SDC. The effect of Ni on the cathode performance is also investigated by impedance spectra analysis.",

keywords = "Dry-pressing, Nickel/ceria catalyst, Perovskite oxide, Symmetrical solid oxide fuel cells, Wet impregnation",

author = "Xingbao Zhu and Zhe L{\"u} and Bo Wei and Xiqiang Huang and Yaohui Zhang and Wenhui Su",

year = "2011",

month = jan,

day = "15",

doi = "10.1016/j.jpowsour.2010.07.055",

language = "英语",

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T1 - A symmetrical solid oxide fuel cell prepared by dry-pressing and impregnating methods

AU - Zhu, Xingbao

AU - Lü, Zhe

AU - Wei, Bo

AU - Huang, Xiqiang

AU - Zhang, Yaohui

AU - Su, Wenhui

PY - 2011/1/15

Y1 - 2011/1/15

N2 - In this study, a simple and cost-effective dry-pressing method has been used to fabricate a symmetrical solid oxide fuel cell (SOFC) where the dense yttria-stabilized zirconia (YSZ) electrolyte film is sandwiched between two symmetrical porous YSZ layers in which La0.75Sr0.25Cr 0.5Mn0.5O3-δ (LSCM) based anode and cathode are incorporated using wet impregnation techniques. The maximum power densities (Pmax) of a single cell with 32 wt.% LSCM impregnated YSZ anode and cathode reach 333 and 265 mW cm-2 at 900 °C in dry H2 and CH4, respectively. The cell performance is further improved with additional impregnation of a small amount of Sm-doped CeO 2 (SDC) or Ni. When 6 wt.% Ni as catalyst is added to both the anode and cathode, Pmax values of 559 and 547 mW cm-2 can be achieved, which are better than with SDC. The effect of Ni on the cathode performance is also investigated by impedance spectra analysis.

AB - In this study, a simple and cost-effective dry-pressing method has been used to fabricate a symmetrical solid oxide fuel cell (SOFC) where the dense yttria-stabilized zirconia (YSZ) electrolyte film is sandwiched between two symmetrical porous YSZ layers in which La0.75Sr0.25Cr 0.5Mn0.5O3-δ (LSCM) based anode and cathode are incorporated using wet impregnation techniques. The maximum power densities (Pmax) of a single cell with 32 wt.% LSCM impregnated YSZ anode and cathode reach 333 and 265 mW cm-2 at 900 °C in dry H2 and CH4, respectively. The cell performance is further improved with additional impregnation of a small amount of Sm-doped CeO 2 (SDC) or Ni. When 6 wt.% Ni as catalyst is added to both the anode and cathode, Pmax values of 559 and 547 mW cm-2 can be achieved, which are better than with SDC. The effect of Ni on the cathode performance is also investigated by impedance spectra analysis.

KW - Dry-pressing

KW - Nickel/ceria catalyst

KW - Perovskite oxide

KW - Symmetrical solid oxide fuel cells

KW - Wet impregnation

UR - https://www.scopus.com/pages/publications/77956874068

U2 - 10.1016/j.jpowsour.2010.07.055

DO - 10.1016/j.jpowsour.2010.07.055

M3 - 文章

AN - SCOPUS:77956874068

SN - 0378-7753

VL - 196

SP - 729

EP - 733

JO - Journal of Power Sources

JF - Journal of Power Sources

IS - 2

ER -

A symmetrical solid oxide fuel cell prepared by dry-pressing and impregnating methods

Abstract

UN SDGs

Keywords

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